Single-Atom Detection
- 1 January 1981
- journal article
- Published by SAGE Publications in Applied Spectroscopy
- Vol. 35 (1) , 1-14
- https://doi.org/10.1366/0003702814731923
Abstract
An overview is presented of the principles and achievements of various laser-assisted detection techniques that have been developed to observe a single or a small number of neutral atoms in the gaseous state. Possible applications of these single-atom detection (SAD) techniques and their significance for the improvement of analytical detection limits are mentioned. Section I describes the general implications of SAD techniques and contains statistical expressions for the mean and the fluctuation of the signal. An intrinsic limit of detection is defined that relates to the statistical fluctuation of the number of registered atoms in the observation volume. Section II gives a classification and a more detailed description of reported techniques. Experimental detection limits are compared with the intrinsic limits predicted by theory. In Section III, conclusions are drawn about the state-of-the-art and suggestions are made for further improvements, including the lowering of the analytical detection limit.Keywords
This publication has 44 references indexed in Scilit:
- Resonance ionization spectroscopy of lithiumOptics Communications, 1979
- Sub-Poissonian photon statistics in resonance fluorescenceOptics Letters, 1979
- Photon-burst method in high-resolution laser spectroscopyPhysical Review A, 1979
- Laser-Enhanced Ionization for Trace Metal Analysis in FlamesPublished by American Chemical Society (ACS) ,1978
- Analytical Chemistry: Using Lasers to Detect Less and LessScience, 1978
- Measuring the velocity of individual atoms in real timeOptics Letters, 1978
- Single-atom detection by SONRESIEEE Journal of Quantum Electronics, 1978
- Simultaneous Observations of Stimulated Raman Scattering and Stimulated Collision-Induced FluorescencePhysical Review Letters, 1977
- Opto-galvanic detection of species in flamesJournal of the American Chemical Society, 1976
- Saturation spectroscopy in molecular iodine by intermodulated fluorescenceOptics Communications, 1972