Impulsive pump-probe and photon-echo spectroscopies of dye molecules in condensed phases
- 1 December 1990
- journal article
- Published by American Physical Society (APS) in Physical Review A
- Vol. 42 (11) , 6920-6923
- https://doi.org/10.1103/physreva.42.6920
Abstract
A theory for impulsive resonant pump-probe and photon-echo spectroscopies of polyatomic dyes in solution is developed. A multimode calculation in which the intramolecular and solvation modes are modeled as Brownian oscillators is presented. Electronic dephasing, the time-dependent Stokes shift, and quantum beats are analyzed.Keywords
This publication has 16 references indexed in Scilit:
- Evolution of the vibronic absorption spectrum in a molecule following impulsive excitation with a 6 fs optical pulseChemical Physics Letters, 1989
- Femtosecond photon echoes from molecules in solutionPhysical Review Letters, 1989
- Theory of quantum beats in optical transmission-correlation and pump-probe experiments for a general Raman configurationPhysical Review A, 1988
- Resonant impulsive-stimulated Raman scattering on malachite greenPhysical Review A, 1988
- Optical Stark Effect in Organic Dyes Probed with Optical Pulses of 6-fs DurationPhysical Review Letters, 1988
- Femtosecond optical Kerr studies on the origin of the nonlinear responses in simple liquidsIEEE Journal of Quantum Electronics, 1988
- Impulsive stimulated light scattering. II. Comparison to frequency-domain light-scattering spectroscopyThe Journal of Chemical Physics, 1987
- Impulsive stimulated light scattering. I. General theoryThe Journal of Chemical Physics, 1987
- Spectral hole burning in large molecules probed with 10 fs optical pulsesChemical Physics Letters, 1986
- Femtosecond Relaxation Dynamics of Large MoleculesPhysical Review Letters, 1986