Photon antibunching in the fluorescence of a single dye molecule trapped in a solid
- 7 September 1992
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 69 (10) , 1516-1519
- https://doi.org/10.1103/physrevlett.69.1516
Abstract
The correlation between fluorescence photons emitted by an optically pumped single molecule of pentacene in a p-terphenyl host has been investigated at short times. The correlation function shows photon antibunching, a unique feature of a nonclassical radiation field, which decreases if two molecules rather than one are pumped at the same time. The peculiarities of the correlation function for a three-level molecule are discussed and the theoretical description outlined.Keywords
This publication has 16 references indexed in Scilit:
- Optical modification of a single impurity molecule in a solidNature, 1992
- Fluorescence spectroscopy and spectral diffusion of single impurity molecules in a crystalNature, 1991
- Single pentacene molecules detected by fluorescence excitation in ap-terphenyl crystalPhysical Review Letters, 1990
- Laser experiments with single atoms as a test of basic physicsIEEE Journal of Quantum Electronics, 1988
- Laser Spectroscopy of Trapped Atomic IonsScience, 1987
- Nonclassical radiation of a single stored ionPhysical Review Letters, 1987
- Macroscopic quantum jumps in a single atomPhysical Review A, 1986
- Shelved optical electron amplifier: Observation of quantum jumpsPhysical Review Letters, 1986
- Multiatom and transit-time effects on photon-correlation measurements in resonance fluorescencePhysical Review A, 1978
- Proposal for the measurement of the resonant Stark effect by photon correlation techniquesJournal of Physics B: Atomic and Molecular Physics, 1976