Evidence for the Polymerization of Ethylene Catalyzed by Ti+ in the Gas Phase
- 1 May 1992
- journal article
- Published by American Chemical Society (ACS) in Journal of the American Society for Mass Spectrometry
- Vol. 3 (4) , 464-466
- https://doi.org/10.1016/1044-0305(92)87074-9
Abstract
In this communication, we report the polymerization of ethylene molecules induced by an atomic ion, namely Ti+, in the gas phase. The experiments are performed by using a newly built selected ion drift tube with laser vaporization source apparatus operated at thermal energies. 50 far, up to twenty ethylene molecules are found to react with Ti+, The evidence that a large number of ethylene molecules react with, and become bonded onto, Ti+ at room temperature strongly suggests that Ti+ induces a reaction between the ethylene molecules that leads to the formation of an ethylene polymer.Keywords
This publication has 6 references indexed in Scilit:
- The bonding strength of Ag+(C2H4) and Ag+(C2H4)2 complexesChemical Physics Letters, 1991
- Methane oligomerization in the gas phase by third-row transition-metal ionsJournal of the American Chemical Society, 1991
- Mechanistic and kinetic study of alkane activation by titanium(I) and vanadium(I) in the gas phase. Lifetimes of reaction intermediatesJournal of the American Chemical Society, 1986
- Gas-phase ion-molecule reactions of iron(+) and titanium(+) with alkanesJournal of the American Chemical Society, 1982
- Gas-phase ion chemistry of titanium tetrachloride and methyltitanium chloride (CH3TiCl3). Reaction of CH3TiCl2+ with ethyleneJournal of the American Chemical Society, 1981
- Ion-molecule reactions in mixtures of titanium tetrachloride with olefins in the gas phaseJournal of the American Chemical Society, 1977