Abstract
A stepwise thermal rearrangement of [(η8-C8H8)Zr(Mes)2](Mes = 2,4,6-Me3C6H2) led to the loss of mesitylene and to a dinuclear complex,[(η8-C8H8)2Zr(µ-2,4-Me 2-6CH2C6H2)2], containing two bridging η3-benzylic groups, which further rearranged to a complex containing a bridging mesityl and a bridging alkylidene ligand, as shown by the X-ray analysis on both complexes.

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