The formation of hex-5-enopyranosides and their selective hydrolysis in methylated polysaccharides

Abstract
The introduction of hex-5-enopyranoside residues into methylated acidic polysaccharides is effected by reduction of uronic acid residues, followed by reaction with triphenyl phosphite methiodide, and dehydroiodination. The selective hydrolysis of hex-5-enopyranosidic linkages with characterization of the 6-deoxyglycos-5-uloses thus formed and location of the aglyconic hydroxyl groups thus exposed has been demonstrated for methylated derivatives of birch xylan and gum arabic. The reaction sequence provides a new method for linkage analysis of acidic polysaccharides.

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