Calculation of photoemission from atoms subject to intense laser fields
- 1 April 1992
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review A
- Vol. 45 (7) , 4998-5010
- https://doi.org/10.1103/physreva.45.4998
Abstract
We use a nonperturbative method to solve the time-dependent Schrödinger equation for an electronic state of an atom subject to a very intense (> W/) laser. The oscillating, time-dependent dipole induced by the laser serves as a source for the photoemission. Calculations of single-atom photospectra reveal peaks at the odd harmonics of the incident laser field superimposed on a broad continuous background. We discuss a series of calculations for the hydrogen atom and a short-range Yukawa potential containing a variable number of bound states. At intensities up to a few times W/ at 1064 nm, we achieve stable, converged spectra that agree very well with previously published results. As the intensity increases to W/, the ionization rate increases to about 1% of the laser frequency, and converged results become extremely difficult to obtain, even for impractically large integration volumes. These difficulties are caused by a rising background due to electron density far from the nucleus and the increasing importance of the interaction of the wave function with the edges of the grid. We discuss the implications of our findings for calculations at high intensity and suggest alternative ways to calculate harmonic emission rates in the strong-ionization regime.
Keywords
This publication has 32 references indexed in Scilit:
- Simple calculations on two-colour multiphoton ionizationJournal of Physics B: Atomic, Molecular and Optical Physics, 1991
- Higher-order harmonic generation in xenon at 1064 nm: The role of phase matchingPhysical Review Letters, 1991
- Coherent soft-x-ray generation by the harmonics of an ultrahigh-power KrF laserPhysical Review A, 1991
- Atomic hydrogen irradiated by a strong laser field: Sturmian basis calculations of rates for high-order multiphoton ionization, Raman scattering, and harmonic generationJournal of the Optical Society of America B, 1990
- Multiphoton processes in an intense laser field: Harmonic generation and total ionization rates for atomic hydrogenPhysical Review A, 1989
- Generation of Optical Harmonics by Intense Pulses of Laser RadiationJournal of Modern Optics, 1989
- Multiple-harmonic generation in rare gases at high laser intensityPhysical Review A, 1989
- Nonlinear Light Scattering Accompanying Multiphoton IonizationPhysical Review Letters, 1989
- Studies of multiphoton production of vacuum-ultraviolet radiation in the rare gasesJournal of the Optical Society of America B, 1987
- Enhancement of high optical harmonics by excess-photon ionisationJournal of Physics B: Atomic and Molecular Physics, 1987