Measurements of Excited-State Population Ratios of Atomic Hydrogen Produced by Charge-Exchange Neutralization of Energetic Proton Beams

Excited-state population ratios for atomic hydrogen have been measured for energetic hydrogen ions neutralized by charge exchange with a number of different metallic vapors and permanent gases. Electric field ionization techniques were used to determine excitation ratios. Detection of the energetic ions and neutrals was accomplished using partially depleted surface-barrier detectors. Counting, using phase-detection techniques in which an add-subtract scaler was phased to the signal, provided an improved signal-to-noise ratio. Two methods were used to provide desired targets. Metallic vapor and permanent-gas thin targets of the order of ${10}^{-5\mathrm{}}$ mTorr cm were produced as chopped neutral beams, using conventional crossed-beam techniques. Gas cells were used to extend these measurements with permanent gases to targets up to seven orders of magnitude thicker. In the latter case, the ion beam was interrupted electrically. Targets investigated were magnesium, potassium, barium, hydrogen, nitrogen, thallium, Freon, water vapor, ammonia, and perfluorodimethylcyclohexane (${\mathrm{C}}_8$ ${\mathrm{F}}_{16}$).