12.3-minCf256and 43-minMd258and systematics of the spontaneous fission properties of heavy nuclides

Abstract
The new isotope 12.3-min Cf256 was produced via the Cf254(t,p) reaction, and a new 43-min isomer of Md258 was produced via the Es255(α,n) reaction. The fragment mass and kinetic energy distributions from the spontaneous fission of Cf256 were found to be very similar to those from the spontaneous fission of lighter Cf isotopes. The mass division is primarily asymmetric, and the average total kinetic energy is 189.8±0.9 MeV. The 43-min Md258 presumably decays by electron capture and provides an opportunity to study the mass and kinetic energy distributions from the spontaneous fission of the 380-μs Fm258 daughter. The observed narrow, symmetric mass distribution and the most probable total kinetic energy of 238±3 MeV are similar to those reported for the spontaneous fission of Fm259 but show a sharp increase in symmetric mass division and total kinetic energy compared to Fm257 and the lighter Fm isotopes. No such abrupt change in properties was observed for Cf256, which, like Fm258, has 158 neutrons. The marked difference between the spontaneous fission properties of the heavier Fm isotopes and those of other spontaneously fissioning nuclides is compared to some theoretical predictions.