Abstract
Self‐consistent field calculations using an optimized minimum basis set of Slater orbitals were carried out for BH3NH3 in order to compute the barrier to internal rotation and its derivatives (changes in the barrier caused by variation of the molecular geometry). In principle both the barrier and its derivatives can be determined experimentally. In addition, the change in equilibrium geometry as the molecule internally rotates was predicted, as well as the diagonal force constants and the dipole moment and its derivatives.

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