Non‐Blinking Semiconductor Colloidal Quantum Dots for Biology, Optoelectronics and Quantum Optics
- 3 April 2009
- journal article
- research article
- Published by Wiley in Chemphyschem
- Vol. 10 (6) , 879-882
- https://doi.org/10.1002/cphc.200800827
Abstract
Twinkle, twinkle: The blinking of semiconductor colloidal nanocrystals is the main inconvenience of these bright nanoemitters. There are various approaches for obtaining non‐blinking nanocrystals, one of which is to grow a thick coat of CdS on the CdSe core (see picture). Applications of this method in the fields of optoelectronic devices, biologic labelling and quantum information processing are discussed. magnified image The blinking of semiconductor colloidal nanocrystals is the main inconvenience of these bright nanoemitters. For some years, research on this phenomenon has demonstrated the possibility to progress beyond this problem by suppressing this fluorescence intermittency in various ways. After a brief overview on the microscopic mechanism of blinking, we review the various approaches used to obtain non‐blinking nanocrystals and discuss the commitment of this crucial improvement to applications in the fields of optoelectronic devices, biologic labelling and quantum information processing.Keywords
This publication has 47 references indexed in Scilit:
- “Giant” Multishell CdSe Nanocrystal Quantum Dots with Suppressed BlinkingJournal of the American Chemical Society, 2008
- Emission Characterization of a Single CdSe-ZnS Nanocrystal with High Temporal and Spectral Resolution by Photon-Correlation Fourier SpectroscopyPhysical Review Letters, 2008
- Blinking suppression and intensity recurrences in single CdSe-oligo(phenylene vinylene) nanostructures: experiment and kinetic modelNanotechnology, 2007
- Multiexcitons in type-II colloidal semiconductor quantum dotsPhysical Review B, 2007
- Mechanisms of fluorescence blinking in semiconductor nanocrystal quantum dotsThe Journal of Chemical Physics, 2005
- Imaging the Photoionization of Individual CdSe/CdS Core−Shell Nanocrystals on n- and p-Type Silicon Substrates with Thin OxidesThe Journal of Physical Chemistry B, 2004
- Polymorph Selectivity under Nanoscopic ConfinementJournal of the American Chemical Society, 2004
- Near-Complete Suppression of Quantum Dot Blinking in Ambient ConditionsJournal of the American Chemical Society, 2004
- Simple model for the power-law blinking of single semiconductor nanocrystalsPhysical Review B, 2002
- From amplified spontaneous emission to microring lasing using nanocrystal quantum dot solidsApplied Physics Letters, 2002