Effects of surface magnetism on optical second harmonic generation

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Abstract
We report on the first experiments showing the influence of surface magnetization on optical second harmonic generation in reflection at a Fe(110) surface. The magneto-optical Kerr effect modifies the hyperpolarizability of the surface in the optical field, leading to a dependence of the second harmonic yield on the direction of magnetization relative to the light fields. For the clean surface an effect of 25% was determined, which decays exponentially with surface contamination by the residual gas, thus demonstrating the high surface sensitivity of this technique.