Search for a fine structure in theC14decay ofRa222

Abstract
The C14 decay of Ra222 has been reinvestigated, using an 85 MBq activity U230 source radiochemically separated, a Si barrier detector, and a superconducting magnetic spectrometer. In a 16 days counting run, 210 C14 events were recorded. The C14 particles energy value 30.930±0.090 MeV was found and an upper limit b≤2×1012 was estimated for the C14 branching ratio to the Pb208 first excited state; the branching-ratio value to the Pb208 ground state, thus equal to the total branching ratio, was found to be b=λc/λα=(2.31±0.31)×1010.