A Relationship Between Acid Precipitation and Three-Dimensional Transport Associated with Synoptic-Scale Cyclones

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Abstract
Field data collected during APEX (Acid Precipitation Experiment) are used in combination with an isentropic trajectory model to analyze the relationship between acid precipitation and three-dimensional transport associated with cyclonic storms. Data are presented which indicate that high acidity in precipitation is often associated with slow transport speed and elevated SO2 concentrations in the dry air feeding into the precipitating regions. Conversely, low acidity is usually related to rapid transit, descending motion, and transport above the atmospheric boundary layer. The results also show that precipitation in the cold sector of a cyclone (in advance of the surface warm front) is often more acidic than that in other sectors of the storm. Four case studies are included to detail some of these meteorological effects. Abstract Field data collected during APEX (Acid Precipitation Experiment) are used in combination with an isentropic trajectory model to analyze the relationship between acid precipitation and three-dimensional transport associated with cyclonic storms. Data are presented which indicate that high acidity in precipitation is often associated with slow transport speed and elevated SO2 concentrations in the dry air feeding into the precipitating regions. Conversely, low acidity is usually related to rapid transit, descending motion, and transport above the atmospheric boundary layer. The results also show that precipitation in the cold sector of a cyclone (in advance of the surface warm front) is often more acidic than that in other sectors of the storm. Four case studies are included to detail some of these meteorological effects.

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