A NEW BIOLOGICAL TARGET OF FUROCOUMARINS: PHOTOCHEMICAL FORMATION OF COVALENT ADDUCTS WITH UNSATURATED FATTY ACIDS

Abstract
Abstract— Furocoumarins, potent skin therapy and tanning agents, form covalent adducts in a photochemical reaction with unsaturated fatty acids. These adducts and the chemical kinetics of their formation have been characterized by chromatography, isotopic tracers, electronic absorbance and fluorescence spectroscopy and mass spectrometry. Adduct formation does not require oxygen. The quantum yield of adduct formation in ethanol or methanol‐water solutions is comparable to the quantum yield for formation of furocoumarin‐thymine adducts in DNA.

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