Syntheses, Structures, and Solid State Properties of One-Dimensional Halogen-Bridged Ni111−X-Ni111Compounds (X˭Cl and Br)

Abstract
Halogen-bridged linear-chain compounds, {[Ni(R,R-chxn)2X]X2}∞ (X˭C1 and Br), were synthesized and their structures have been determined by low-temperature X-ray diffraction analyses. The novel one-dimensional Ni111 -X-Ni111 structure with no Peierls distortion, which is an extreme limit of the MII -X-MIV mixed-val

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