Abstract
Tetrathiofulvalene derivatives Ia-e reacted with an equimolar amount of 2,3-dichloro-5,6-dicyano-p-benzoquinone (DDQ) in hot acetonitrile or benzene to give new stable cation-radical and anion-radical complexes IIa-e, which had various mole ratios (1:1, 1:2, 2:1).

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