Abstract
The total internal-conversion coefficients have been measured for E2 transitions from first excited state to ground state in five heavy deformed nuclei. α-particle gating was used to determine the population of the first excited levels from parent decays. Photon spectra, as observed by a well-type NaI(Tl) detector in coincidence with the gating α particles, were analyzed to determine the ratio of γ transitions to total transitions. The α gating spectra and photon spectra were analyzed on a computer, when necessary, using a nonlinear least-squares curve-fitting program. The resulting coefficients are 19.6±1.4 for the 84.4-keV transition in Ra224, 158±7 for the 57.6-keV transition in Th228, 780±55 for the 43.5-keV transition in U234, 607±29 for the 45.28-keV transition in U236, and 845±93 for the 42.88-keV transition in Pu240. The internal-conversion coefficient for the transition in Pu240 is somewhat lower than the theoretical predictions of Hager and Seltzer and of Sliv and Band, whereas the internal-conversion coefficient for the transition in U234 is somewhat higher. The internal-conversion coefficients for the remaining transitions agree with the theoretical values within the experimental uncertainties.