Crystal and molecular structure of a novel mixed-spin binuclear nickel(II) complex with N,N′,N″,N‴-tetrakis(2-aminoethyl)-1,4,8,11-tetra-azacyclotetradecane

Abstract
The crystal structure of [Ni2(taec)Cl]Cl3·H2O was determined by the single-crystal X-ray diffraction method, where taec is N,N′,N″,N‴-tetrakis(2-aminoethyl)-1,4,8,11-tetra-azacyclotetradecane. The [Ni2(taec)Cl]3+ cation has a novel binuclear structure in which one of the nickel ions is co-ordinated by a square-planar N4 donor set and the other by a distorted square-pyramidal N4Cl donor set.

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