Dynamics of weakly connected solids: Silica aerogels

Publisher Website
Google Scholar
Abstract
Apply neutron spin-echo spectroscopy, we investigate low-energy vibrational excitations in a series of silica aerogels of varying connectivity. Connectivity is adjusted both by precursor solution chemistry and by heat treatment. Polymeric aerogels show fractonlike densities of states, whereas colloidal materials exhibit a peak in the μev regime. On sintering, the low-frequency excitations disappear. We conclude that neutron spin-echo spectroscopy provides a measure of the topological aspects of disordered materials.

This publication has 13 references indexed in Scilit: