Infrared Spectra of Alkali Metal Azide Crystals

Abstract
The infrared spectra of CsN3, RbN3, KN3, and NaN3 crystals have been recorded at room temperature and at liquid‐nitrogen temperature. Considerable anharmonicity in the fundamentals of N3 − and combinations with lattice modes has been observed. Splitting of the doubly degenerate ν2 has been observed. Discrepancies between the several reported values of ν3 are discussed.

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