Polarized-neutron study of the coherent paramagnetic scattering amplitude of metallic erbium

Abstract
Polarized-neutron techniques have been used to measure the coherent paramagnetic scattering amplitude of high-purity single crystals of metallic erbium at 300 K. The angular dependence of the coherent-scattering amplitude has been determined with the external magnetic field (H=22 kOe) applied parallel as well as perpendicular to the c axis of the crystal. It has been found that the angular dependence of the scattering amplitude for Hc as well as Hc is in good agreement, except at small scattering angles, with the 4f-electron magnetic form factor calculated using relativistic Dirac-Fock wave functions. At small scattering angles the experimental points were found to be systematically higher than the theoretical curves obtained by least-square fitting of the calculated 4f-electron form factor to the large-angle experimental points. This small-angle contribution, attributed to the polarization of the conduction bands of erbium, has an unusual angular dependence; it is different from either a 5d or 6s atomic form factor and exhibits a non-negative oscillatory character.