Abstract
Values of one‐bond J(C35 Cl) and T1(35Cl) were determined for small chlorine‐containing molecules through 13C scalar relaxation in the rotating frame. A method is suggested for evaluating the contribution of scalar relaxation which eliminates experimental imperfections. The magnitude of J(C35Cl) seems to be influenced by the same factors as J(CF) values. The differences in 35Cl relaxation times are rationalized in terms of the molecular reorientation time.

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