Low-temperature magnetic structure ofFeSn2

Abstract
FeSn2 is a collinear antiferromagnet between TN=378 K and Tt=93 K as shown by previous neutron diffraction and Sn119 Mössbauer studies. Below Tt, two different noncollinear antiferromagnetic structures are consistent with neutron diffraction results, one, called structure I, being canted along with c axis and the other, denoted structure II, being canted in the basal plane (001) along the [110] direction of the chemical cell of FeSn2. On the other hand, two magnetic structures canted in the basal plane, IIa and IIb, which differ only in the propagation vector agree with Sn119 Mössbauer spectra. The simultaneous use of the two techniques has allowed an unambiguous choice of structure IIa which is simply characterized by a combination of the magnetic couplings observed in the high-temperature magnetic structures of FeSn2 and MnSn2.

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