Evidence of a large quantum shift of the antiferromagnetic resonance in three quasi-one-dimensional antiferromagnets

Abstract
Antiferromagnetic resonance experiments in three one-dimensional manganese compounds [CsMnCl3′2H2O (CMC), (CH3)2 NH2 MnCl3 (DMMC), and (CH3)4 NMnCl3 (TMMC)] show disagreement with the classical antiferromagnetic resonance theory. In the three compounds we observe a positive shift in magnetic field of the resonance lines corresponding to the low-frequency mode. We show that this shift is larger for the compounds with smaller ratio |JJ| and try to explain this effect in terms of the quantum spin reduction of the magnon energy.