Synthesis of some medium- and large-ring cycloalk-2-ene-1,4-diones by intramolecular coupling of αω-bis-diazoketones

Abstract
In the presence of Cu(acac)2(Hacac = acetylacetone) some αω-bis-diazoketones couple intramolecularly with loss of nitrogen giving cycloalk-2-ene-1,4-diones; the enediones can be converted into fused ring cyclopentenones by successive treatment with sodium dithionite and sodium hydroxide.

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