Chemically induced interface states in photoelectrochemical cells

Abstract
This letter reports for the first time a significant improvement of p-GaP photocathodes for hydrogen evolution by treatment with ruthenium ions. Sub-band-gap spectroscopy has revealed that contrary to expectations the ruthenium treatment introduces new states in the gap 1.23 eV above the valence-band edge and close to a band edge. A new model based upon kinetic considerations is proposed to explain these effects.

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