Variation of chemical shielding with intermolecular interactions and rovibrational motion. I. 19F nuclei in BF3, CF4, SiF4, and SF6

Abstract
The chemical shifts due to rotational and vibrational motion in CF4, SiF4, BF3, and SF6 are obtained by extrapolation of 19F resonance frequencies to zero density. The second virial coefficients of chemical shielding, σ1(T), are obtained at the same time from the slopes. It is found that the σ1 values for these molecules do not depend on temperature nearly as strongly as was previously reported.