Neutron-scattering study of stripe-phase order of holes and spins in
- 1 September 1996
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review B
- Vol. 54 (10) , 7489-7499
- https://doi.org/10.1103/physrevb.54.7489
Abstract
We present a neutron diffraction study of charge and spin order within the planes of , a crystal in which superconductivity is anomalously suppressed. At low temperatures we observe elastic magnetic superlattice peaks of the type (1/2±ε,1/2,0) and charge-order peaks at (2±2ε,0,0), where ε=0.118. After cooling the crystal through the low-temperature-orthorhombic (LTO) to low-temperature-tetragonal (LTT) phase transition near 70 K, the charge-order peaks appear first at ∼60 K, with the magnetic peaks appearing below 50 K. The magnetic peaks increase in intensity by an order of magnitude below 3 K due to ordering of the Nd ions. We show that the observed diffraction features are consistent with stripe-phase order, in which the dopant-induced holes collect in domain walls that separate antiferromagnetic antiphase domains. The Q dependence of the magnetic scattering indicates that the low-temperature correlation length within the planes is substantial (∼170 Å), but only very weak correlations exist between next-nearest-neighbor planes. Correlations between nearest-neighbor layers are frustrated by pinning of the charge stripes to the lattice distortions of the LTT phase. The spin-density-wave amplitude corresponds to a Cu moment of 0.10±0.03 . The behavior of the electrical resistivity within the LTT phase is examined, and the significance of stripe-phase correlations for understanding the unusual transport properties of layered cuprates is discussed. © 1996 The American Physical Society.
Keywords
This publication has 68 references indexed in Scilit:
- Critical Buckling for the Disappearance of Superconductivity in Rare-Earth-DopedPhysical Review Letters, 1994
- Spin structures of tetragonal lamellar copper oxidesPhysical Review Letters, 1994
- Soft phonon behavior and magnetism at the low temperature structural phase transition of La1.65Nd0.35CuO4Zeitschrift für Physik B Condensed Matter, 1993
- Frustrated electronic phase separation and high-temperature superconductorsPhysica C: Superconductivity and its Applications, 1993
- Study on magnetic ordering in (La, Nd, Sr)2CuO4Physica C: Superconductivity and its Applications, 1992
- Lattice instabilities and the effect of copper-oxygen-sheet distortions on superconductivity in dopedPhysical Review B, 1991
- Holes and magnetic textures in the two-dimensional Hubbard modelPhysical Review B, 1991
- Phase separation in at-JmodelPhysical Review B, 1990
- Comparison between muon spin rotation and neutron scattering ttudies on the 3-dimensional magnetic ordering of La2CuO4-yPhysica C: Superconductivity and its Applications, 1988
- Antiferromagnetism inPhysical Review Letters, 1987