Antitumor agents. 25. Synthesis and antitumor activity of uracil and thymine .alpha.-methylene-.gamma.-lactones and related derivatives

Abstract
Uracil and thymine .alpha.-methylene-.gamma.-lactones and related derivatives were synthesized as novel potential alkylating antitumor agents. The synthesis of these compounds involved the convenient Reformatsky type reaction between ethyl .alpha.-(bromomethyl)acrylate and the proper pyrimidinyl ketones. Preliminary in vivo tumor assays indicated that these compounds were active against the Walker 256 carcinosarcoma in rats and the P-388 lymphocytic leukemia as well as the B-16 melanotic melanoma in mice at 2.5-25 mg/kg.

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