Phosphoramides. VII. Phenyl N,N'-Dimethylphosphorodiamidate as a Reagent for Synthesis of 3-Methylthieno[2,3-d]pyrimidin-4(3H)-ones.

Abstract
3-Methylthieno[2,3-d]pyrimidin-4(3H)-ones [with biological and pharmacological activity] (4) were obtained in an exothermic reaction by heating phenyl N,N''-dimethylphosphorodiamidate 1 and methyl 2-acylamino-3-thiophenecarboxylates (3) to 250.degree. C. From 3 where R1.tbd.C6H5, R2.tbd.H and R3.tbd.CH3 the expected 4 in 40% yield was obtained, but 6-methyl-2-phenyl-4-methylaminothieno[2,3-d]pyrimidine was also isolated in 45% yield.

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