Static higher polarizabilities ofH2

Abstract
The higher polarizabilities γzzzz, Bzz:zz, and Czz:zz have been calculated for H2 using different-sized basis sets composed of James-Coolidge basis functions. The most-accurate wave functions led to the values 674, -89.8, and 5.97 a.u., respectively. It is emphasized that these properties are critically sensitive to wave-function quality.

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