A radiological survey was conducted on the undeveloped portions of the site of the former Main Technical Area (TA-1) of the Los Alamos Scientific Laboratory in north-central New Mexico. Between 1943 and 1965, research work on nuclear weapons was carried out in TA-1. The area was decontaminated and demolished in stages, and beginning in 1966 the land was given to Los Alamos County or sold to private interests. The survey disclosed traces of radioactive contamination undetected or considered insignificant during original demolition in the 1950s and 1960s. The remaining contamination was removed in 1975 and 1976 to levels considered to pose no health or safety hazards and, further, to the lowest levels considered practicable. Methods used in the survey included measurement techniques for detecting alpha emitters such as uranium and plutonium, extensive surface and subsurface soil sampling, and use of conventional health physics instrumentation to provide detailed information on approximately 16 hectares (40 acres) of land. As a result of the decontamination efforts, approximately 15,000 m/sup 3/ of contaminated or potentially contaminated material was removed to an approved radioactive waste disposal site on ERDA property. Full details of the methods, findings, decision criteria, and as-left conditions are documented.