Electrohydrodynamic Charge Relaxation and Interfacial Perpendicular-Field Instability

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Abstract
The small‐amplitude motions of a plane interface between two fluids stressed by an initially perpendicular electric field are investigated. The fluids are modeled as Ohmic conductors and the convection of the surface charge caused by the dynamic interplay of interfacial electric shear stresses and the viscous stresses is highlighted. The influence of viscosity on instability growth rates in the zero‐shear stress limits of perfectly conducting and perfectly insulating interfaces is described and compared to cases involving electrical shear stresses. Detailed attention is given to the instability of an interface between fluids having electrical relaxation times long compared to times of interest. It is shown that, for many common liquids, even a slight amount of surface charge makes the interface unstable at a considerably lower voltage than would be expected from theories based on the dielectrophoretic limit of no interfacial free charge. Experiments, performed using high‐frequency ac stresses, gradually increased dc fields, and abruptly applied dc fields, support the theoretical model. In the general case, the electric Hartmann number is identified as an index to the dominance of the electric shear stresses over the viscous shear stresses in determining the interfacial convection of free charge.