Solid-liquid transitions in argon clusters

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Abstract
The solid-liquid transitions in argon clusters of medium size (N>55) are studied by molecular dynamics simulations on a cluster of 79 atoms. Over an intermediate range of total energy, the cluster exhibits a ‘‘dynamical coexistence’’ of solid and liquid states, in which the cluster fluctuates between solid and liquid states. We propose that for medium-sized clusters, the existence of two types of structures, low-energy solid and high-energy liquid structures, leads to the dynamical coexistence. We predict that the dynamical coexistence is a finite-size effect of a bulk melting transition.

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