11.5% solar conversion efficiency in the photocathodically protected p-InP/V3+-V2+-HCI/C semiconductor liquid junction cell

Abstract
Oxidation of the surface of p‐InP with alkaline peroxide and treatment with dilute potassium cyanide increase the efficiency of the p‐InP/V2+−V3+ ‐HCl/C cell to 11.5%. The open circuit voltage of the cell follows the redox potential of the solution over a 0.5 V range. The lack of voltage pinning is consistent with photoemission studies of Spicer e t a l., showing that adsorption of oxygen on p‐InP raises the surface fermi level from a position near the valence band maximum to noe near the conduction band minimum.

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