Abstract
Reaction of [(ML2Cl)2] with Tl[9-SMe2-nido-7.8-C2B9H10] affords the new compounds [3,3-L2-4-SMe2-closo-3,1,2-MC2B9H10]. Compounds 1(M = Rh, L = CO), 2(M = Rh, L222-1,5-C8H12) and 3(M = Pd, L22, σ-5OMe-C8H12) were characterised by microanalysis, multinuclear NMR spectroscopy and, in the case of 1 and 2, single-crystal X-ray diffraction studies. The experimentally determined conformations of the ML2 fragments relative to the carbaborane ligands in 1 and 2 are in broad agreement with those predicted by analysis of the results of extended Hückel molecular orbital (EHMO) calculations on model compounds, especially in the case of 2. Reaction of 3 with HBF4 in diethyl ether affords the cationic heteroborane [3-(η22-1,5-C8H12)-4-SMe2-closo-3,1,2-PdC2B9H10]+4+. Crystallographic study of 4+BF4 reveals a molecular conformation substantially influenced by H F inter-ion contacts. Comparative EHMO calculations on 2 and 4+ imply that the majority of the additional positive charge in the latter is not localised on the pendant sulfur atom alone, but rather is delocalised over the 12 cluster vertices and the atoms directly bonded to them.

This publication has 0 references indexed in Scilit: