Spin Liquid State in an Organic Mott Insulator with a Triangular Lattice

Abstract
H1 NMR and static susceptibility measurements have been performed in an organic Mott insulator with a nearly isotropic triangular lattice, κ(BEDTTTF)2Cu2(CN)3, which is a model system of frustrated quantum spins. The static susceptibility is described by the spin S=1/2 antiferromagnetic triangular-lattice Heisenberg model with the exchange constant J250K. Regardless of the large magnetic interactions, the H1 NMR spectra show no indication of long-range magnetic ordering down to 32 mK, which is 4 orders of magnitude smaller than J. These results suggest that a quantum spin liquid state is realized in the close proximity of the superconducting state appearing under pressure.
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