Repulsive van der Waals and Dipole-Quadrupole Interaction in the Excited LiCs Molecule

Abstract
The authors report strong repulsive van der Waals and dipole-quadrupole interactions in the Σ and Π potentials of the LiCs molecule dissociating into Li 2P and Cs 6S atoms. Theoretical results derived from second-order perturbation theory are verified by investigating experimentally the wavelength dependence of the quasistatic wings of the Li resonance lines broadened by Cs ground-state atoms.

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