Ab initio calculation of orthogonal parameters for complex configurations using B-splines

Abstract
An ab initio second-order calculation of the parameter values corresponding to the five orthogonal two-electron operators which can describe the term structure of a pd configuration to infinite order has been carried out for the 2p3d configuration in O III. The second-order contributions to the parameters from eight single and double excitations have been calculated including the contributions from all bound and continuum states.

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