Abstract
A single-crystal X-ray analysis of Co(paphy)Cl2 is reported. The complex crystallises as green, monoclinic needles: space group P21/c; a= 8·72, b= 11·93, c= 14·32 Å, β= 119·1°, Z= 4. A least-squares refinement of positional and anisotropic vibrational parameters of all 18 atoms has allowed the R factor for 1257 Weissenberg intensities to converge at 8·9%. The complex consists of monomeric molecules with a five-co-ordinate stereo-chemistry for which a square pyramidal description is preferred. Isomorphism with Co(paphy)Br2 and with halogeno-2,2′,2″-terpyridyl complexes of Mn, Co, Ni, Cu, and Zn indicates that these compounds should be similarly described.

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