Über Naphtho[1.8-de]-1,3-dioxine / Naphtho[1,8-de]-1,3-dioxines

Abstract
Treatment of 1,8-Dihydroxy-naphthaline with bromochloromethane/K3CO3 in DMF gives Naphtho[1,8-de]-1,3-dioxine (1a) in good yield. The bromo (1b) and nitro compound (1c) can be obtained free of isomorics by electrophilic substitution of la. Bromolithium exchange of 1b leads to a lithium organic compound, which possibles the synthesis of alkyl-, olefinic-, and carboxylic derivatives of the substrate 1a. In a similar way the treatment of 2,3-dihydroxynaphthazarin with chlorobromomethane/K2CO3 gives the naphtho[1,8-de;4,5-d′e′]-bis-1,3-dioxine (3a). The substrate 3a can be subjected to electrophilic aromatic substitutions.

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