The Electronic Structure and the He(I) Photoelectron Spectrum of Tricarbonylcyclooctatetraene-iron [1]

Abstract
The highest occupied molecular orbitals of tricarbonylcyclooctatetraene-iron (1) have been derived from those of tricarbonyl-butadiene-iron and butadiene. Based on this MO diagram and an INDO-type calculation the He(I) photoelectron (PE) spectrum of 1 could be interpreted. Using the ⊿ SCF and the transition operator method (TOM) the first five bands of the PE spectrum of 1 could be assigned.

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