Abstract
Force constants have been calculated for Se8 (α-monoclinic selenium) after reassigning the literature values of the fundamental frequencies and using a modified Urey-Bradley force field with six force constants. Very good agreement between observed and calculated frequencies was obtained and valence force constants were calculated. A non-linear relationship holds for SeSe stretching force constants and bond distances. Using the Se8 force constants the fundamental frequencies of the square-planar Se4 2+ were calculated and compared with the observed values

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