F+centre in (Ca-Sr) carbonated hydroxyapatites

Abstract
Powdered samples of synthetic carbonated hydroxyapatites with variable amounts of strontium substituting for calcium, obtained by precipitation, were studied by ESR at the X-band frequencies after heating at 400°C for 24 h, X-irradiation and annealing at 150°C for 30 min. The F+ centre spectrum exhibiting orthorhombic symmetry was recorded between RT and 120 K, with <g>≃2. When the amount of carbonate inside the samples increases, the spectral intensity has the same behaviour than that of the quantity of O2- vacancies calculated from results of chemical analysis. Our results are a confirmation of the existence of two different mechanisms of charge compensation when CO3 2- substitutes for PO4 3-, and they also show that Sr ions are not located in cation sites adjacent to carbonate ions.

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