Fluxional dirhodium complexes: crystal and molecular structure of [Rh2(CO)2(µ-SPh)2(C8H8)]

Abstract
Variable temperature n.m.r. studies of complexes [Rh2(CO)2(µ-SPh)2L] and [Rh2(µ-SR)2L2](R = Me, Et, Pri, But, or Ph; L = cyclo-octatetraene or cyclo-octa-1,5-diene) reveal the existence of both an olefin rotation and an inversion of non-planar Rh2S2 ring; this non-planarity is established by an X-ray diffraction study of [Rh2(CO)2(µ-SPh)2(C8H8)].

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