Paramagnetic-Resonance Absorption in the Optically Populated StateF522,E52ofTm2+in CaF2

Abstract
Paramagnetic-resonance absorption was observed in the metastable state F522, E52 of CaF2:Tm2+ which was populated by an optical source. The measured g value of 1.453±0.002 can be compared with the calculated value of (-) 1.478. The g discrepancy of 0.025 is the same as found for the ground state. From the hyperfine constant for two values of J, a core-polarization correction of (+) 14±3 Mc/sec is derived for the ground state.

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