Pressure-Induced Phase Transitions in Triplet-Exciton Crystals

Abstract
The pressure dependence of the exchange‐narrowed triplet‐exciton magnetic resonance in (φ3PCH3)+‐(TCNQ)2 and (φ3AsCH3)+(TCNQ)2 has been observed at 170 Mc/sec in the ranges 1–9 kbar, and 220°—362°K. Pressure‐induced phase transitions in these salts are reported. The observed p—T phase diagram for (φ3AsCH3)+(TCNQ)2 can be explained remarkably well in terms of an elementary theory of non‐interacting triplet excitons.

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