Convenient syntheses of bifunctional C12-acyclic compounds from cyclododecanone

Abstract
The conversion of cyclododecanone by convenient, non-hazardous, and high-yielding reactions into a set of useful C12-bifunctional intermediates is described. Baeyer–Villiger oxidation and hydrolysis give a hydroxy acid, successively converted into the bromo acid, bromo alcohol, crude bromo aldehyde, pure bromo aldehyde ethylene acetal, and pure bromo aldehyde. Preferred reagents for the transformation CO2H → CHO are borane–dimethyl sulphide followed by dimethyl sulphoxide–oxalyl dichloride–triethylamine.

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