Measurement of high-order optical nonlinear susceptibilities in semiconductor-doped glasses

Abstract
The optical susceptibilities of CdSxSe1−x ‐doped glasses were observed up to χ(11) using a spatially resolved phase‐matched multiwave mixing technique. Using a pulsed dye laser tuned near the band gap, measurements were performed for ‖χ(3)‖, ‖χ(5)‖, and ‖χ(7)‖ in four different commercial filter glasses.